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Article

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Title

Improving the Impact Strength and Heat Resistance of 3D Printed Models: Structure, Property, and Processing Correlationships during Fused Deposition Modeling (FDM) of Poly(Lactic Acid)

Authors

[ 1 ] Instytut Technologii Materiałów, Wydział Budowy Maszyn i Zarządzania, Politechnika Poznańska | [ P ] employee

Scientific discipline (Law 2.0)

[2.8] Materials engineering

Year of publication

2018

Published in

ACS Omega

Journal year: 2018 | Journal volume: vol. 3 | Journal number: no. 4

Article type

scientific article

Publication language

english

Keywords
EN
  • 3D printing
  • biopolymers
  • crystallinity
  • organic polymers
  • plastics
Abstract

EN A fused deposition modeling method was used in this research to investigate the possibility of improving the mechanical properties of poly(lactic acid) by changing the thermal conditions of the printing process. Sample models were prepared while varying a wide range of printing parameters, including bed temperature, melt temperature, and raster angle. Certain samples were also thermally treated by annealing. The prepared materials were subjected to a detailed thermomechanical analysis (differential scanning calorimetry, dynamic mechanical analysis, heat deflection temperature (HDT)), which allowed the formulation of several conclusions. For all prepared samples, the key changes in mechanical properties are related to the content of the poly(lactic acid) crystalline phase, which led to superior properties in annealed samples. The results also indicate the highly beneficial effect of increased bed temperature, where the best results were obtained for the samples printed at 105 °C. Compared to the reference samples printed at a bed temperature of 60 °C, these samples showed the impact strength increased by 80% (from 35 to 63 J/m), HDT increased by 20 °C (from 55 to 75 °C), and also a significant increase in strength and modulus. Scanning electron microscopy observations confirmed the increased level of diffusion between the individual layers of the printed filament.

Date of online publication

23.04.2018

Pages (from - to)

4400 - 4411

DOI

10.1021/acsomega.8b00129

URL

https://pubs.acs.org/doi/abs/10.1021/acsomega.8b00129

License type

ACS AuthorChoice License

Open Access Mode

open journal

Open Access Text Version

final published version

Date of Open Access to the publication

at the time of publication

Ministry points / journal

15

Ministry points / journal in years 2017-2021

15

Impact Factor

2,584

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