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Article

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Title

Interfacial insights into the polarization protocol - towards reducing corrosion and improving the cycle life of electrochemical capacitors

Authors

[ 1 ] Instytut Chemii i Elektrochemii Technicznej, Wydział Technologii Chemicznej, Politechnika Poznańska | [ P ] employee

Scientific discipline (Law 2.0)

[7.6] Chemical sciences

Year of publication

2024

Published in

ACS Applied Materials & Interfaces

Journal year: 2024 | Journal volume: vol. 16 | Journal number: iss. 21

Article type

scientific article

Publication language

english

Keywords
EN
  • corrosion
  • current collectors
  • energy storage devices
  • stainless steel
  • supercapacitors
Abstract

EN The number of scientific publications on the impact of corrosion on current collectors on the working parameters of electrochemical capacitors is very limited. The aim of current research is to search for new, environmentally friendly chemical power sources and energy storage devices and to improve existing ones. Therefore, this article presents a simple and effective way to improve the life of a symmetric electrochemical capacitor by changing the direction of electrode polarization, which in turn inhibits the corrosion of the current collector. This slows the degradation of current collectors of positive electrode over long durations. However, activated carbon electrode corrosion also occurs. Experiments on capacitors with stainless steel and gold current collectors indicate that the lifespan of the latter is much longer than that of the former. Therefore, current collector corrosion has a distinct and detrimental impact on electrochemical capacitor operation. Moreover, the research results indicate that carbon corrosion results from current collector corrosive damage.

Pages (from - to)

27242 - 27253

DOI

10.1021/acsami.4c00767

URL

https://pubs.acs.org/doi/10.1021/acsami.4c00767

License type

CC BY (attribution alone)

Open Access Mode

czasopismo hybrydowe

Open Access Text Version

final published version

Date of Open Access to the publication

at the time of publication

Full text of article

Download file

Access level to full text

public

Ministry points / journal

200

Impact Factor

8,3 [List 2023]

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